High levels of black carbon found at remote site in Siberia

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(Phys.org)—A team of researchers with members from Sweden, the U.S., Russia, Norway and Austria has found higher than expected levels of black carbon at a remote test site in Siberia. In their paper published in Proceedings of the National Academy of Sciences, the team describes the amount of black carbon they found and its sources.

Black carbon consists of that are small enough to become airborne. One such example is soot sent into the air from burning coal. It is not a greenhouse gas, but does contribute to global warming via another means. It lands on top of snow, and because it is black, absorbs heat from the sun, which causes two problems—one is that some of that in the northern latitudes, which would normally be reflected back into the atmosphere, remains on the ground. The other is that it contributes to higher than normal snow melt. In this new effort, the research team ventured into a remote part of Siberia to gather statistics on levels, because it is one of the few northern places left on Earth where data regarding its presence is not regularly collected.

The team set up a research station just outside of the town of Tiksi and immediately began monitoring the amount of black carbon that landed on its sensors. They report that they found more than was expected and that it was coming from an unexpected source. The biggest source, they found, was automobile exhaust, which was surprising because there is very little automobile traffic in Siberia. They suggest it likely traveled from more populous places in Europe, Russia and China. Before arriving at the site, the researchers had suspected that the biggest source would be gas flares caused by the oil industry, which are common in Siberia.

The researchers were able to identify the source of the black carbon by looking at its isotopic fingerprint—different sources produce different isotopes. Regular black soot, for example, has very little carbon 14. Such testing revealed that coal burning was the second largest source of black carbon in the region, though they noted things changed by season—during the summer, burning biomass was the biggest source.

The researchers suggest that it is important that all sources of climate change be accounted for if accurate predictions and models are to be made—a critical factor for figuring out how to reverse what is occurring.

More information: Patrik Winiger et al. Siberian Arctic black carbon sources constrained by model and observation, Proceedings of the National Academy of Sciences (2017). DOI: 10.1073/pnas.1613401114

Abstract
Black carbon (BC) in haze and deposited on snow and ice can have strong effects on the radiative balance of the Arctic. There is a geographic bias in Arctic BC studies toward the Atlantic sector, with lack of observational constraints for the extensive Russian Siberian Arctic, spanning nearly half of the circum-Arctic. Here, 2 y of observations at Tiksi (East Siberian Arctic) establish a strong seasonality in both BC concentrations (8 ng⋅m−3 to 302 ng⋅m−3) and dual-isotope–constrained sources (19 to 73% contribution from biomass burning). Comparisons between observations and a dispersion model, coupled to an anthropogenic emissions inventory and a fire emissions inventory, give mixed results. In the European Arctic, this model has proven to simulate BC concentrations and source contributions well. However, the model is less successful in reproducing BC concentrations and sources for the Russian Arctic. Using a Bayesian approach, we show that, in contrast to earlier studies, contributions from gas flaring (6%), power plants (9%), and open fires (12%) are relatively small, with the major sources instead being domestic (35%) and transport (38%). The observation-based evaluation of reported emissions identifies errors in spatial allocation of BC sources in the inventory and highlights the importance of improving emission distribution and source attribution, to develop reliable mitigation strategies for efficient reduction of BC impact on the Russian Arctic, one of the fastest-warming regions on Earth.

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